Éditeur(s) : Copernicus Gesellschaft Mbh
Résumé : During the GWADASEIS cruise (Lesser Antilles volcanic arc, February-March 2009) a very high resolution (VHR) seismic-reflection survey was performed in order to constrain Late Quaternary to Present faulting. The profiles we obtained evidence frequent "ponding" of reworked sediments in the deepest areas, similar to the deposition of Mediterranean "homogenites". These bodies are acoustically transparent (few ms t.w.t. thick) and are often deposited on the hanging walls of dominantly normal faults, at the base of scarps. Their thickness appears sufficient to compensate (i.e. bury) co-seismic scarps between successive earthquakes, resulting in a flat and horizontal sea floor through time. In a selected area (offshore Montserrat and Nevis islands), piston coring (4 to 7m long) was dedicated to a sedimentological analysis of the most recent of these particular layers. It corresponds to non-stratified homogenous calcareous silty sand (reworked calcareous plankton and minor volcanoclastics). This layer can be up to 2 m thick, and overlies fine-grained hemipelagites. The upper centimeters of the latter represent the normal RedOx water/sediment interface. Pb-210 and Cs-137 activities lack in the massive sands, while a normal profile of unsupported Pb-210 decrease is observed in the hemipelagite below, together with a Cs-137 peak corresponding to the Atmospheric Nuclear Experiments (1962). The RedOx level was thus capped by a recent instantaneous major sedimentary event considered as post-1970 AD; candidate seismic events to explain this sedimentary deposits are either the 16 March 1985 earthquake or the 8 October 1974 one (M-w = 6.3 and M-w = 7.4, respectively). This leads to consider that the syntectonic sedimentation in this area is not continuous but results from accumulation of thick homogenites deposited after the earthquakes (as observed in the following weeks after Haiti January 2010 event, McHugh et al., 2011). The existence of such deposits suggests that, in the area of study, vertical throw likely results from cumulated effects of separated earthquakes rather than from aseismic creep. Examination of VHR profiles shows that all major co-seismic offsets are recorded in the fault growth sequence and that co-seismic offsets can be precisely estimated. By using a sedimentation rate deduced from Pb-210 decrease curve (0.5 mmyr(-1)) and taking into account minor reworking events detected in cores, we show that the Redonda system may have been responsible for five > M-6 events during the last 34 000 yr. The approach presented in this work differs from fault activity analyses using displaced sets of isochronous surfaces and postulating co-seismic offsets. Combining VHR seismic imagery and coring we can decipher co-seismic vs. slow continuous displacement, and thus actually estimate the amplitude and the time distribution of major co-seismic offsets.
Natural Hazards And Earth System Sciences (1561-8633) (Copernicus Gesellschaft Mbh), 2012 , Vol. 12 , N. 5 , P. 1755-1767

Droits : Author(s) 2012. CC Attribution 3.0 License.
http://archimer.ifremer.fr/doc/00089/20040/21990.pdf
DOI:10.5194/nhess-12-1755-2012
http://archimer.ifremer.fr/doc/00089/20040/

Éditeur(s) : HAL CCSD Elsevier
Résumé : While most rocks from active volcanoes display ((210)pb/Ra-226) activity ratios lower than or close to the equilibrium value of 1, several other have ratios much higher than 1. Transfer of Rn-222 by magmatic volatiles has often been advocated to explain both Pb-210 deficits and excesses. We develop here a model to account for Pb-210 excesses through Rn-222 accumulation. We show that large Pb-210 excesses can be readily obtained, even for moderate ratios of degassing magma over accumulating magma, in a closed-system model where the Rn-222 atoms produced by decay of Ra-226 in the degassing magma are continuously extracted by a gas phase. For a given duration of volatile transfer, relative Pb-210 excesses are expected to be much larger than Pb-210 deficits. This model is applied to samples from Santorini (Aegean arc) and Surtsey (Iceland) both of which show high ((210)pb/Ra-226) ratios of 6.7 and 2.3 respectively at the time of eruption. The agreement with field data suggests that Rn-222 accumulation leading to Pb-210 excesses might be a rather common process in zoned magma chambers as well as in individual lava flows, and that it can be described by a closed-system model.
ISSN: 0012-821X

hal-00496398
https://hal.archives-ouvertes.fr/hal-00496398
DOI : 10.1016/j.epsl.2010.02.048

Éditeur(s) : HAL CCSD Elsevier
Résumé : Finding records of past catastrophic storm events is essential to evaluate the long term climatic evolution in a given coastal area. This question has been addressed by the study of sediment cores sampled in a small coastal lagoon of the French Mediterranean coast (Pierre Blanche lagoon). Two cores were studied in detail and revealed the presence of three main storm events. The sedimentation rates calculated using the CFCS Pb-210 model, in agreement with Cs-137 data, are 3 +/- 0.4 and 4.2 +/- 0.7 mm y(-1) near the border and in the center of the lagoon respectively. This suggests that the 0.6 m deep lagoon could be filled with sediments over the next 150 yr. Our study shows that storm events can be characterized in sedimentary sequences identified by facies, grain size and faunal assemblages (lagoonal and marine species). Comparison of Pb-210, C-14 chronology and historical accounts suggest that the three identified storm events took place in 1742, 1839 and 1893 A.D. (i.e. about one catastrophic event per century).
ISSN: 0025-3227

hal-00411189
https://hal.archives-ouvertes.fr/hal-00411189
DOI : 10.1016/j.margeo.2008.03.001

Éditeur(s) : HAL CCSD University of Arizona
Résumé : International audience
Taiwan is a young and seismically active mountain belt, where a series of strong earthquakes (M>7) have occurred over the past hundred years. Identifying historical earthquakes around Taiwan is a key to better constrain the geodynamic of this active region. Sedimentological and geochemical analyses of surface sediments from one station offshore east Taiwan revealed the presence of coarse-grained layers interpreted as turbidites. The age of these layers have been determined by 210Pb, 137Cs, and 241Am chronology. Dating of the three most recent turbidites provides ages of AD 2001±3, AD 1950±5, and AD 1928±10. The results show striking temporal correspondence of turbidite layers to large (M≥6.8) earthquakes recorded in the region since the 20th century. The chronologies of sediment layers lead us to believe that turbidites resulted from the 2003 Taitung earthquake (M 6.8), the 1951 Chengkong earthquake (M 7.1), and the 1935 Lutao earthquake (M 7.0), respectively. Such a good correlation between turbidites and high-magnitude (M≥6.8) historical and instrumental seismic events suggests that turbidite paleoseismology constitutes a valuable tool for earthquake assessment in the eastern Taiwan margin. Moreover, the modern reservoir radiocarbon age and the regional marine reservoir correction (ΔR) of the Kuroshio Current off Taiwan were estimated by comparing accelerator mass spectrometry (AMS) 14C ages with ages derived from corrected 210Pb profiles and historical accounts of identifiable seismic events. Such a determination is important to calibrate the 14C ages of marine materials for accurate comparison of marine and continental geological records. Our calculated mean ΔR value of 232±54 14C yr (n=2) is higher than its modern value of 86±40 14C yr. This high value can be explained by the presence of local upwelling cells and turbulence in the Kuroshio Current, north of Green Island. These upwelling cells bring 14C-depleted water to the surface, resulting in an increase of the modern ΔR value in this portion of the Kuroshio Current.
ISSN: 0033-8222

hal-01306986
https://hal.archives-ouvertes.fr/hal-01306986
DOI : 10.1017/RDC.2015.3

Éditeur(s) : HAL CCSD Copernicus Publications on behalf of the European Geosciences Union
Résumé : International audience
During the GWADASEIS cruise (Lesser Antilles volcanic arc, February–March 2009) a very high resolution (VHR) seismic-reflection survey was performed in order to constrain Late Quaternary to Present faulting. The profiles we obtained evidence frequent " ponding " of reworked sediments in the deepest areas, similar to the deposition of Mediterranean " homogenites ". These bodies are acoustically transparent (few ms t.w.t. thick) and are often deposited on the hanging walls of dominantly normal faults, at the base of scarps. Their thickness appears sufficient to compensate (i.e. bury) co-seismic scarps between successive earthquakes, resulting in a flat and horizontal sea floor through time. In a selected area (offshore Montserrat and Nevis islands), piston coring (4 to 7 m long) was dedicated to a sedimento-logical analysis of the most recent of these particular layers. It corresponds to non-stratified homogenous calcareous silty sand (reworked calcareous plankton and minor volcanoclas-tics). This layer can be up to 2 m thick, and overlies fine-grained hemipelagites. The upper centimeters of the latter represent the normal RedOx water/sediment interface. 210 Pb and 137 Cs activities lack in the massive sands, while a normal profile of unsupported 210 Pb decrease is observed in the hemipelagite below, together with a 137 Cs peak corresponding to the Atmospheric Nuclear Experiments (1962). The RedOx level was thus capped by a recent instantaneous major sedimentary event considered as post-1970 AD; candidate seismic events to explain this sedimentary deposits are either the 16 March 1985 earthquake or the 8 October 1974 one (M w = 6.3 and M w = 7.4, respectively). This leads to consider that the syntectonic sedimentation in this area is not continuous but results from accumulation of thick homogen-ites deposited after the earthquakes (as observed in the following weeks after Haiti January 2010 event, McHugh et al., 2011). The existence of such deposits suggests that, in the area of study, vertical throw likely results from cu-mulated effects of separated earthquakes rather than from aseismic creep. Examination of VHR profiles shows that all major co-seismic offsets are recorded in the fault growth sequence and that co-seismic offsets can be precisely estimated. By using a sedimentation rate deduced from 210 Pb decrease curve (0.5 mm yr −1) and taking into account minor reworking events detected in cores, we show that the Redonda system may have been responsible for five > M 6 events during the last 34 000 yr. The approach presented in this work differs from fault activity analyses using displaced sets of isochronous surfaces and postulating co-seismic offsets. Combining VHR seismic imagery and coring we can decipher co-seismic vs. slow continuous displacement, and thus actually estimate the amplitude and the time distribution of major co-seismic offsets.
Natural Hazards and Earth System Science

insu-01585969
https://hal-insu.archives-ouvertes.fr/insu-01585969
https://hal-insu.archives-ouvertes.fr/insu-01585969/document
https://hal-insu.archives-ouvertes.fr/insu-01585969/file/nhess-12-1755-2012-beck.pdf
DOI : 10.5194/nhess-12-1755-2012

Éditeur(s) : EDP Sciences
Résumé : We present results obtained from a pristine site of French Guiana (South America), at the Pic Matecho, a region far from gold mining activity. This area contains a small permanent lake, a rare situation in French Guiana. Tree canopy, soils and Lake Matecho sediments were analysed in total Hg and Pb-210. The annual deposit of litterfall is estimated at 40 mug (Hg)/m(2)/y. The top sediment content of 0.2 mug (Hg)/g indicates a large contribution of the atmospheric deposit. In sediment, the decrease of total Hg with depth is neither due to local human influence, nor to increase of atmospheric background during this century. It is attributed to remineralization of organic matter in the upper part of the sediment : the majority of the total Hg deposited at the water/sediment interface is not permanently trapped in the sediment but remobilized in water. Interpretation of the historical sediment profile suggests a constant deposit rate over the last millennium.
Journal De Physique Iv (1155-4339) (EDP Sciences), 2003-05 , Vol. 107 , P. 859-862

Droits : 2003 EDP Sciences
http://archimer.ifremer.fr/doc/00000/10630/9348.pdf
DOI:10.1051/jp4:20030433
http://archimer.ifremer.fr/doc/00000/10630/

Éditeur(s) : HAL CCSD Elsevier
Résumé : Several nuclides of the ;238;U (;234;U, ;230;Th, ;226;Ra, ;210;Pb) and ;235;U (;231;Pa, ;227;Ac) decay series have been measured through gamma spectrometry in the U-bearing episyenites of the Bernardan mine (northwest Massif Central, France), in order to study recent mobilizations in the U-deposit and their time-scales. (;230;Th/;238;U) and (;231;Pa/;235;U) ratios show that U has been little affected during the last 350 ky, especially in the U-rich samples. In contrast, ;226;Ra was subjected to a general redistribution, with a clear tendency for Ra to be lost from the U-rich samples and added to U-poor samples. The highest Ra excesses are present in low-U samples, and are related to adsorption onto iron hydroxides. Ra appears to have been redistributed within the mineralised episyenitic bodies, which seem to remain in ;226;Ra–;238;U radioactive equilibrium, a result consistent with the earlier study of Leroy [1984. Episyénitisation dans le gisement d'uranium du Bernardan (Marche): Comparaison avec des gisements similaires du Nord-Ouest du Massif Central français. Miner. Depos. 19, 26–35]. As shown by the ;226;Ra and ;210;Pb data, the Ra redistribution was very active between 8 and 0.1 ky, and this might be a consequence of the hydrological changes in groundwater circulation accompanying the Holocene climate warming.
ISSN: 0009-2541

hal-00407600
https://hal.archives-ouvertes.fr/hal-00407600
DOI : 10.1016/j.chemgeo.2007.06.020

Éditeur(s) : HAL CCSD Elsevier
Résumé : International audience
Excess gas phase in magmas erupting explosively is well known worldwide. However, the origin of this gas phase, in excess of what can be dissolved in the erupting magma at depth, and the rate of gas accumulation is less well defined. The 2010 mildly explosive eruption at Eyjafjallajökull, Iceland, produced mingled tephra of benmoreitic and trachytic composition whereas alkali basalt was emitted during preceding flank eruption. Tephra of the first explosive phase are composed of three glass types, alkaline rhyolite, mixed benmoreite, and basalt, which suggests that the basaltic magma intruded a pre-existing rhyolitic magma chamber, and ultimately triggered the eruption. The mixed benmoreitic tephra (erupted on 15 and 17 April 2010) had large 210Po in excess of 210Pb View the MathML source[(Po210/Pb210)0=1.88] at the time of eruption, and possibly a small 210Pb excess over its parent 226Ra. In contrast, the preceding flank eruption produced basalt with View the MathML source(Po210)0=0, upon eruption, and the final trachyte had lost most of its 210Po during open-system degassing. The 210Po excess in the first erupted benmoreites is interpreted to result from 210Po degassing of basaltic magma and the accumulation of 210Po-enriched gas, either in the upper part of the basaltic intrusion, below the rhyolite–basalt interface, or in the pre-existing residual rhyolitic magma chamber. From a simple model of radon and polonium accumulation in the rhyolitic reservoir, the ratio of the mass of basalt magma degassing over the mass of magma accumulating the excess gas decreased from 20 to 15 over 2 days, implying zoned magma reservoir, with the uppermost and gas-richest part erupting first. The duration of pre-eruptive gas accumulation in this model is approximately one year. This corresponds closely to the initiation of a seismic swarm beneath Eyjafjallajökull, early June 2009, which was the first pre-eruptive signal detected. The coincidence between initiation of gas accumulation at relatively shallow depth and deeper seismicity strongly suggests that the excess gas phase originated from a basalt magma batch intruded at depth, and that this gas phase reached the surface approximately a year later.
ISSN: 0012-821X

hal-01217142
https://hal.archives-ouvertes.fr/hal-01217142
DOI : 10.1016/j.epsl.2015.06.054

Éditeur(s) : HAL CCSD Elsevier
Résumé : International audience
The present study reports data on CO2-rich geothermal waters and their associated carbonate deposits from the SW part of the Permian Lodève Basin (South of France). Both waters and carbonates are enriched in 226Ra, with activities up to 2.2 Bq/L and 3.5 Bq/g respectively. A series of carbonate samples precipitated around the studied wells since 1990 were dated through the 226Ra-210Pb and 228Ra-228Th methods, and the results are discussed in a new Concordia diagram. While both methods give comparable dates for many samples, Ra-Pb ages are sometimes much older than Ra-Th ages. We propose that these discrepancies result from the adsorption of 222Rn daughter nuclides in such a Rn-rich environment. The (228Ra/226Ra)0 activity ratios calculated at the time of deposition are remarkably constant for about 12 years, suggesting the presence of a steady-state aquifer. The low (228Ra/226Ra)0 ratios (0.348 ± 0.008) are best explained if most of the Ra derives from the Cambrian carbonate series (mainly dolostone) underlying the Permian Basin, which have low Th/U and similar (228Ra/226Ra) ratios. This study suggests that Ra and other alkaline-earth elements do not necessarily originate from the rocks surrounding the deep geothermal reservoir, but rather may be introduced into the CO2-rich water during its transfer towards the surface and interaction with carbonate rocks.
ISSN: 0009-2541

hal-01053715
https://hal.archives-ouvertes.fr/hal-01053715
DOI : 10.1016/j.chemgeo.2014.02.008

Éditeur(s) : HAL CCSD Société géologique de France
Résumé : International audience
The central part of the Gulf of Lions shoreline is characterized by many coastal wetlands that resulted from the interaction between a process of shoreline regularization by migrations of littoral barriers and a slow filling of the back-barrier areas by the riverine and marine inputs. Analyses of Late-Holocene deposits with a very high-resolution multi-proxy study of two sediment cores, allow us to reconstruct the evolution of this coastal system. Two main Holocene sediment units are identified overlying a Pliocene carbonate continental formation. The lower unit consists of sandy and pebbly marine sediments deposited around 7800 B.P., during the final stand of the last sea level rise. Just above, the upper unit displays lagoonal grey clay silts with shells and some intercalated layers of silty sands related to paleostorm events. The age model was established from radiocarbon dating, for the oldest part of the core. Over the last century, sedimentation rates were calculated using the CFCS Pb-210 model, together with Cs-137 data. Radiocarbon data show an increase in he accumulation rate from the base to the top of cores. Marine sand units related to the last transgressive deposit allow to refine the curve of Holocene post-glacial sea level rise. Sedimentological and faunal analyses associated with chronological data provide a means for reconstructing the Late-Holocene paleoenvironments along this part of the coast and suggest that the final closure of the coastal lagoon by the sandy barrier occurred at around 730 +/- 120 yr cal B.P. The beginning of this closure, together with the progradation of the coastal plain, could be responsible for the decline in economic activity of the Lattara harbour during the Roman period.
La partie centrale du littoral du golfe du Lion est caractérisée par de nombreuses lagunes qui résultent de l'interaction entre un processus de régularisation du trait de côte par migration de barrières littorales et d'un lent remplissage des zones situées en arrière des barrières par des apports continentaux et marins. Les analyses des dépôts tardi-holocènes avec une étude multi-traceurs à très haute résolution de deux carottes sédimentaires nous permettent de reconstruire l'évolution de ce système côtier. Deux unités sédimentaires holocènes sont identifiées recouvrant une formation pliocène carbonatée. L'unité inférieure est constituée de sables et de galets d'origine marine déposés vers 7800 B.P., durant les stades ultimes de la dernière remontée marine. Audessus, l'unité supérieure montre des dépôts d'argile et de silt gris coquilliers d'origine lagunaire, dans lesquels sont intercalés des niveaux de sable silteux révélant la présence d'événements de tempêtes. Le modèle d'âge est établi à partir de dates radiocarbones pour les parties les plus anciennes des archives sédimentaires, tandis que pour le dernier siècle, les taux de sédimentation sont calculés en utilisant le modèle CFCS pour le 210Pb, associé aux données de 137Cs. Les données 14C montrent une augmentation du taux d'accumulation depuis la base jusqu'en surface des carottes. Les unités de sables marins liées aux dépôts de la dernière transgression marine permettent de préciser la courbe post-glaciaire de remontée du niveau marin. Les analyses sédimentologiques et faunistiques associées aux données chronologiques fournissent une méthode permettant de reconstituer les paléoenvironnements littoraux tardi-holocènes dans la zone d'étude et suggèrent que la fermeture finale de ces lagunes par le cordon sableux survient autour de 730 ± 120 ans cal B.P. Le début de cette fermeture, associée à la une progradation deltaïque, pourrait être responsable du déclin des activités économiques du port de Lattara durant la période Romaine.
EISSN: 1777-5817

halshs-00740923
https://halshs.archives-ouvertes.fr/halshs-00740923
DOI : 10.2113/gssgfbull.181.1.27

Éditeur(s) : HAL CCSD Elsevier
Résumé : International audience
The eastern margin of the Tibetan Plateau is a key region to understand the formation and tectonic evolution of the plateau. Most studies concentrated on the Longmen Shan range that corresponds to the tectonically very active boundary between the Tibetan Plateau and the Sichuan Basin. This work addresses the deformation and exhumation pattern in the poorly understood metamorphic Danba dome situated at the conjunction between the southern Longmen Shan range and the major strike-slip Xian Shui He fault. The Early Mesozoic and Cenozoic evolution of the dome are then compared to the regional evolution of eastern Tibet. The about 830 Ma zircon U–Pb ages obtained on the Gezong and Gongcai gneiss as well as U–Pb ages on inherited zircons in the Early Mesozoic granites confirm the occurrence of Neo-Proterozoic magmatic episodes in the Danba basement at 800–900 Ma and 650–750 Ma. Following the closure of the Palaeotethys Ocean, granitoids were emplaced in the Danba metamorphic basement and Triassic cover from about 230 Ma to about 170 Ma. The western part of the Lian He Kau granitic massif, emplaced (between 210 and 200 Ma) within the Triassic cover sequence of the dome was only slightly affected by the Early Mesozoic deformation. However, in the eastern, deeper level compartment of the massif, ductile deformation occurred between 200 and 190 Ma, contemporaneous with the onset of the Barrovian-type metamorphism dated at 200–180 Ma. That deformation is compatible with the Early Mesozoic deformation observed in the Longmen Shan range and with the development of the large-scale décollement level in the Songpan Garzê area. Apatite fission track data then indicate that, following the Oligocene–Middle Eocene onset of eastward motion of the Songpan Garzê terrane, the Danba dome developed as a crustal-scale antiform during the Late Miocene–Early Pliocene (10–4 Ma). The exhumation was controlled by the Lian He Kau fault (a major transpressive structure parallel to the Xian Shui He fault) and the associated Manai thrust faults. Regionally, while the Oligocene–Middle Miocene exhumation phase seems to have been of regional extent, the Late Miocene to Present day phase is localised along the Longmen Shan range thrusts as well as along the back-thrusts formed by the Lian He Kau, Manai and associated faults.
ISSN: 0743-9547

insu-01117657
https://hal-insu.archives-ouvertes.fr/insu-01117657
DOI : 10.1016/j.jseaes.2015.02.009

Éditeur(s) : HAL CCSD Elsevier
Résumé : International audience
This article summarizes the geodynamic evolution of the Variscan to Mesozoic Tethyan subduction history, based on a review of geochronological data from Eastern Anatolia and the Lesser Caucasus, and new isotopic ages for the Georgian crystalline basements. The geological history of the basements of Georgia (Transcaucasus) and NE Turkey (eastern Pontides) appears to be similar and provides evidence for a continuously active continental margin above a north-dipping subduction since at least the Lower Jurassic. New La-ICPMS U-Pb ages from the Georgian basement provide further evidence for the derivation of the Transcaucasus and its western continuation (the eastern Pontides) from Gondwana. A migmatized granodiorite provides preserved magmatic zircon cores with an age of 474 ± 3 Ma, while the age of migmatization is constrained by its 343 ± 2 Ma metamorphic rims. Metamorphism is synchronous with widespread I-type granites that were emplaced at 335 ± 8 Ma in the neighbouring Dzirula massif, and in the eastern Pontides. These U-Pb ages are in close agreement with recently obtained Ar/Ar ages from biotites and muscovites from metamorphic schists and U-Pb ages ranging from 340 to 330 Ma in the Georgian basement. The narrow range of ages suggests that the Variscan LP-HT metamorphic event in the eastern Pontides and Georgia was of short duration and likely related to mantle-derived intrusives. Furthermore, we suggest that (1) rifting of the Pontides-Transcaucasus block (PTB) from Gondwana at 450–350 Ma could have been driven by roll-back of the south-dipping Rheic slab, (2) that the main metamorphic and coeval magmatic events are related to the accretion of the PTB to the Eurasian margin at c. 350 Ma, while the source of magmatism is ascribed to slab detachment of the south-dipping slab at 340 Ma and that (3) three subduction zones may have been contemporaneously active in the Tethyan domain during the Jurassic: (i) the Lesser Caucasus South Armenian Block (SAB) shares a similar Gondwana affinity, but bears younger ages for its MP-MT metamorphic evolution and calc-alkaline magmatism bracketed from 160 to 123 Ma; (ii) north-dipping subduction below the PTB from c. 210 Ma to 150 Ma; (iii) northward intra-oceanic subduction bracketed from 180 to 90 Ma between the SAB and the PTB.
ISSN: 0264-3707

hal-01347761
https://hal.archives-ouvertes.fr/hal-01347761
DOI : 10.1016/j.jog.2016.03.003

Éditeur(s) : HAL CCSD Elsevier
Résumé : International audience
We present in this study the first data on Ra isotopes, 222Rn, and 210Pb in waters from the Lez karst system, one of the main ground-water resources in the South of France. The low Ra isotope activities of the Lez system waters (from 0.35 to 3.45 mBq/L of 226Ra) were measured by gamma spectrometry using the method developed in our previous work. Our data reveal the coherent behavior of 226Ra in Lez spring waters, well correlated to other major and trace elements, like Cl, Na, K, Mg, Li, Rb and Ba. The (228Ra/226Ra) ratios are distinct between the Lez spring (0.60 to 0.72) and two neighboring springs (0.52 to 0.65), showing the spatial variability in karst systems. In spite of their small variations in the Lez spring, it was possible to trace different water components and mixing processes from Lower-Cretaceous, Upper-Jurassic and Middle Jurassic end-members, in agreement with previous studies based on major and trace elements. Data obtained on waters derived from the Upper-Jurassic karst reveal that their (228Ra/226Ra) ratios are not related to the Th/U ratio of the Jurassic limestone, but are rather influenced by the soil and alterite cover of the recharge area.222Rn activities in the Lez spring are relatively low (0.5 to 3.7 Bq/L) compared to other karst regions. The highest 222Rn activities are found in diluted waters following heavy rainfall episodes, suggesting a subsurface origin of Rn. Soil and alterite samples that have much higher 226Ra activities (from 51 to 130 Bq/kg), compared to those from the main aquifer rocks (from 2.9 to 16 Bq/kg), are probably the main source of Rn, rather than the rocks of the karst itself. The study of several flood episodes reveals the correlation between Rn peak-values or total activity discharged at the spring with cumulative rainfall. Finally, 222Rn dissolved in water decays to 210Pb, and our data show that constraints on transfer times of underground waters can potentially be obtained from their coupled measurement.
ISSN: 0009-2541

hal-01622749
https://hal.archives-ouvertes.fr/hal-01622749
DOI : 10.1016/j.chemgeo.2017.06.022