Éditeur(s) : HAL CCSD IOP Publishing
Résumé : Radioactive pollutants are naturally present in microelectronic device materials and can be an issue for the reliability of devices. The main concern is alpha emitters that produce high-energy particles (a few MeV) that ionize the semiconductor and then trigger soft errors. The question is to know what kinds of radionuclides are present in the device, their location in the device and the abundance of each species. In this paper we describe tools that are required to address the issue of radioactive pollutants in electronic devices.
ISSN: 0268-1242

hal-01504448
https://hal.archives-ouvertes.fr/hal-01504448
DOI : 10.1088/1361-6641/aa5479

Éditeur(s) : Elsevier
Résumé : A study of organic carbon mineralization from the Congo continental shelf to the abyssal plain through the Congo submarine channel and Angola Margin was undertaken using in situ measurements of sediment oxygen demand as a tracer of benthic carbon recycling. Two measurement techniques were coupled on a single autonomous platform: in situ benthic chambers and microelectrodes, which provided total and diffusive oxygen uptake as well as oxygen microdistributions in porewaters. In addition, sediment trap fluxes, sediment composition (Org-C, Tot-N, CaCO3, porosity) and radionuclide profiles provided measurements of, respectively input fluxes and burial rate of organic and inorganic compounds. The in situ results show that the oxygen consumption on this margin close to the Congo River is high with values of total oxygen uptake (TOU) of 4 +/- 0.6, 3.6 +/- 0.5 mmol m(-2) d(-1) at 1300 and 3100m depth, respectively, and between 1.9 +/- 0.3 and 2.4 +/- 0.2 mmol m(-2) d(-1) at 4000 m depth. Diffusive oxygen uptakes (DOU) were 2.8 +/- 1.1, 2.3 +/- 0.8, 0.8 +/- 0.3 and 1.2 +/- 0.1 mmol m(-2) d(-1), respectively at the same depths. The magnitude of the oxygen demands on the slope is correlated with water depth but is not correlated with the proximity of the submarine channel-levee system, which indicates that cross-slope transport processes are active over the entire margin. Comparison of the vertical flux of organic carbon with its mineralization and burial reveal that this lateral input is very important since the sum of recycling and burial in the sediments is 5-8 times larger than the vertical flux recorded in traps. Transfer of material from the Congo River occurs through turbidity currents channelled in the Congo valley, which are subsequently deposited in the Lobe zone in the Congo fan below 4800 m. Ship board measurements of oxygen profiles indicate large mineralization rates of organic carbon in this zone, which agrees with the high organic carbon content (3%) and the large sedimentation rate (19 mm y(-1)) found on this site. The Lobe region could receive as high as 19 mol C m(-2) y(-1), 1/3 being mineralized and 2/3 being buried and could constitute the largest depocenter of organic carbon in the South Atlantic.
Deep Sea Research Part II: Topical Studies in Oceanography (0967-0645) (Elsevier), 2009-11 , Vol. 56 , N. 23 , P. 2223-2238

Droits : 2009 Elsevier B.V. All rights reserved.
http://archimer.ifremer.fr/doc/2009/publication-7316.pdf
DOI:10.1016/j.dsr2.2009.04.005
http://archimer.ifremer.fr/doc/00000/7316/

Éditeur(s) : HAL CCSD Elsevier
Résumé : International audience
11 4 : CEA/HC 12 13 Corresponding author: 14 pierre.legoff@cea.fr -+333 80 23 40 00 -+333 80 23 52 09 15 16 Abstract 17 As one of the three natural isotopes of hydrogen, tritium is ubiquitous and might potentially 18 be present in any water or organic molecule that constitutes a biological matrix. Milk is one of 19 the most frequently monitored foodstuffs in the vicinity of chronic release of radionuclides, as 20 it is a very common product and also because it integrates deposition on large areas of grass at 21 a local scale. Different parameters have been studied to assess their impact on the reliability 22 of tritium measurements. The volume of the sample, the technique used to extract the water 23 and the level of dehydration modulate the results but in different ways: dispersion of results, 24 under-or overestimation of the tritium activity. The influence of sample storage and 25 preparation has also been investigated. Methodological improvements of tritium 26 measurements in the free water of milk are proposed. 27 28
ISSN: 0265-931X

hal-01117741
https://hal.archives-ouvertes.fr/hal-01117741
https://hal.archives-ouvertes.fr/hal-01117741/document
https://hal.archives-ouvertes.fr/hal-01117741/file/Tritium%20in%20the%20free%20water%20of%20milk-FINAL.pdf
DOI : 10.1016/j.jenvrad.2013.09.006

Éditeur(s) : Pergamon-elsevier Science Ltd
Résumé : The environment is impacted by natural and anthropogenic disturbances that occur at different spatial and temporal scales, and that lead to major changes and even disequilibria when exceeding the resiliency capacities of the ecosystem. With an annual mean flow of 1700 m(3) s(-1), the Rhone River is the largest of the western Mediterranean basin. Its annual solid discharges vary between 2 and 20 Mt, with flood events responsible for more than 70% of these amounts. In the marine coastal area, close to the mouth, both flocculation and aggregation lead to the formation of fine-grained deposits, i.e. the prodelta. This area is characterized by sediment accumulation rates up to 20-50 cm yr(-1) and high accumulations of particle reactive contaminants such as various man-made radionuclides released into the river by nuclear facilities or arising form prior atmospheric nuclear tests (1954-1980) and the Chernobyl accident (April 1986). This prodelta, however, cannot be considered as a permanent repository for particle reactive pollutants since it is subjected to reworking processes. Sediment dynamics had to be linked to the influences of hydrodynamic and atmospheric events such as high flow rates or storms close to the Rhone River mouth. An experiment was carried out during the winter 2006 based on the deployment of two ADCPs and six altimeters at the Grand Rhone mouth for several months. This type of installation has never been used before in this area because of the hard meteorological conditions and the strong fishing activities. However, results showed pluricentimetric rises of the sedimentary level just after river flood events and decreases during storms, generated by southeast winds. Radiotracers and grain size depth profiles helped to characterise the studied events and to establish inventories of sediments and radionuclides. A cruise (CARMEX) was carried out during this same period to collect water samples, suspended particles and sediment cores. The results enabled us to link both river flow and wind characteristics to events recorded on the sea floor, i.e. resuspension, accumulation, consolidation, etc. Deposits of 11 cm of sediments were estimated during flood periods and bottom shear stresses up to 5 N m(-2) were calculated during sediment erosion phases. (C) 2010 Elsevier Ltd. All rights reserved.
Continental Shelf Research (0278-4343) (Pergamon-elsevier Science Ltd), 2010-05 , Vol. 30 , N. 9 , P. 1095-1107

Droits : 2010 Elsevier B.V. All rights reserved.
http://archimer.ifremer.fr/doc/00006/11695/8479.pdf
DOI:10.1016/j.csr.2010.02.015
http://archimer.ifremer.fr/doc/00006/11695/

Éditeur(s) : HAL CCSD Elsevier
Résumé : International audience
Numerous field studies highlighted the capacities of marine sponges to bioaccumulate trace elements and assessed their potential as biomonitors of the marine environment. Experimental works demonstrated that dissolved metals and radionuclides can be taken up directly by sponge tissues but, to the best of our knowledge, little is known on the contribution of the dietary pathway through the consumption of contaminated bacteria considered as one of the trophic source in sponge diet. Objectives of this work are to study trophic transfer of radiotracers 110mAg, 241Am, 109Cd, 57Co, 134Cs, 54Mn and 65Zn from the marine bacteria Pseudomonas stutzeri to the Mediterranean sponges Aplysina cavernicola and Ircinia oros. P. stutzeri efficiently bioaccumulated trace elements in our culture experimental conditions with CF comprised between 105 and 107 after 48 hours of growth in radiolabeled medium. When fed with these radiolabelled bacteria, A. cavernicola took up around 60% of radiotracers accumulated in trophic source except 134Cs for which only 8% has been transferred from bacteria to sponge. Contrasting to this, I. oros retained only 7% of 110mAg, 109Cd and 65Zn counted in bacteria, but retained 2-fold longer accumulated metals in its tissues. The sponge inter-specific differences of accumulation and depuration following a trophic exposure are discussed with respect to the structure and the clearance capacities of each species.
ISSN: 0045-6535

hal-01217273
https://hal.archives-ouvertes.fr/hal-01217273
https://hal.archives-ouvertes.fr/hal-01217273/document
https://hal.archives-ouvertes.fr/hal-01217273/file/Pub%20Bacteria%20CHEM_HAL.pdf
DOI : 10.1016/j.chemosphere.2015.10.046

Éditeur(s) : HAL CCSD Elsevier
Résumé : Among the radionuclides that can migrate from radioactive wastes buried within consolidated argillaceous rocks, I-129 poses a particular problem due to its high mobility in geomedia and its very long half-life of 1.6 10(7) years. Previous studies carried out on such rocks showed the existence of a low iodide retardation regarding the other anion species. The purpose of the present study was two-fold. It was hoped (1) to confirm this retardation by means of radial diffusion experiments and (2) to estimate the influence of the initial iodide concentrations towards the iodide uptake. The results obtained from in-diffusion stage show that (1) no iodide uptake occurs at high initial concentrations and (2) an uptake at low initial concentrations cannot be clearly evidenced. Finally. the most singular behaviour of iodide was highlighted for all the initial iodide concentrations, from the out-diffusion stage. during which some amount of iodide, available for out-diffusion, were not involved in the diffusion process. Although the origin of such phenomenon remains unclear, a kinetic effect for the iodide uptake was proposed, assuming that the period of 55days (corresponding to the in-diffusion stage duration) would be necessary for inducing the iodide uptake. This kinetic effect, already shown elsewhere by (Descostes. M., Blin, V., Bazer-Bachi, F., Meier, P., Grenut, B., Radwan. J., Schlegel, M.L., Buschaert, S.. Coelho, D, Tevissen, E. Diffusion of anionic species in Callovo-Oxfordian argillites and Oxfordian limestones. In press for Appl. Geochem.) on similar materials, needs to be deepened.
ISSN: 0079-1946

hal-00412393
https://hal.archives-ouvertes.fr/hal-00412393
DOI : 10.1016/j.pce.2008.05.020

Éditeur(s) : HAL CCSD Elsevier
Résumé : International audience
The dating of alluvial landforms by cosmogenic nuclides requires distinguishing the pre-deposition inheritance from the post-deposition history of the clasts in the studied marker. Moreover, estimating catchment-scale erosion rates from the concentrations of cosmogenic nuclides in active alluvia requires a good knowledge of the local/regional relationships between rock exhumation and transport through space and time. This is still poorly known for timescales of tens of thousand years. In order to document the evolution of clast exhumation and transport rates through time, we analyze in situ 10Be concentrations in boulders and cobbles from hillslopes to outlet of an arid mountainous catchment located in Gobi-Altay, Mongolia, strongly affected by global climatic changes during the Pleistocene-Holocene period. Samples were collected on bedrock, abandoned alluvial deposits, active colluvia and alluvia. Our results show a large 10Be scattering in the active river bed, consistent with a low and discontinuous catchment erosion rate dominated by mass wasting and fluvial incision. On the contrary, pre-exposure signal within abandoned terraces is much more homogeneous, consistent with climatic pulses responsible of strong erosional events on hillslopes and rapid fluvial transport. These results show that exhumation/transport processes at the catchment scale vary in style and intensity through time as a consequence of climatic oscillations. The occurrence of abrupt climatic changes during short periods of time recorded by 10Be concentrations in abandoned alluvia raise questions about the temporal applicability of catchment erosion rates derived from cosmogenic nuclide concentrations measured in sediments of active rivers. On the other hand, strong and short erosion events limit and homogenize the pre-exposure 10Be signal in associated deposits like debris-flows, making them particularly suitable markers for dating in active tectonic and paleoclimatic studies.
ISSN: 0169-555X

hal-00626702
https://hal.archives-ouvertes.fr/hal-00626702
https://hal.archives-ouvertes.fr/hal-00626702/document
https://hal.archives-ouvertes.fr/hal-00626702/file/GEOMOR-2485R1_corrected.pdf
DOI : 10.1016/j.geomorph.2011.07.023

Éditeur(s) : HAL CCSD Elsevier Masson
Résumé : International audience
o abstract
ISSN: 0761-8425

hal-01187123
https://hal-univ-rennes1.archives-ouvertes.fr/hal-01187123
DOI : 10.1016/j.rmr.2015.06.015